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4-hydroxy-3-methylbenzonitrile

Product Name
4-hydroxy-3-methylbenzonitrile
CAS No.
15777-70-5
Chemical Name
4-hydroxy-3-methylbenzonitrile
Synonyms
2-Methyl-4-cyanophenol;4-hydroxy-3-methylbenzonitrile;Benzonitrile, 4-hydroxy-3-methyl-
CBNumber
CB41559556
Molecular Formula
C8H7NO
Formula Weight
133.15
MOL File
15777-70-5.mol
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4-hydroxy-3-methylbenzonitrile Property

Melting point:
93-95 °C
Boiling point:
180-182 °C(Press: 12 Torr)
Density 
1.17±0.1 g/cm3(Predicted)
storage temp. 
Inert atmosphere,Room Temperature
pka
8.19±0.18(Predicted)
Appearance
Light brown to yellow Solid
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Safety

HS Code 
2926907090
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Hazard and Precautionary Statements (GHS)

Symbol(GHS)
Signal word
Warning
Hazard statements

H302Harmful if swallowed

H315Causes skin irritation

H319Causes serious eye irritation

H335May cause respiratory irritation

Precautionary statements

P261Avoid breathing dust/fume/gas/mist/vapours/spray.

P305+P351+P338IF IN EYES: Rinse cautiously with water for several minutes. Remove contact lenses, if present and easy to do. Continuerinsing.

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N-Bromosuccinimide Price

TRC
Product number
H972700
Product name
4-Hydroxy-3-methylbenzonitrile
Packaging
250mg
Price
$75
Updated
2021/12/16
AK Scientific
Product number
J96889
Product name
4-Hydroxy-3-methylbenzonitrile
Packaging
5g
Price
$330
Updated
2021/12/16
AK Scientific
Product number
J96889
Product name
4-Hydroxy-3-methylbenzonitrile
Packaging
10g
Price
$500
Updated
2021/12/16
Apolloscientific
Product number
OR908148
Product name
4-Hydroxy-3-methylbenzonitrile
Purity
98%
Packaging
5g
Price
$646
Updated
2021/12/16
Apolloscientific
Product number
OR908148
Product name
4-Hydroxy-3-methylbenzonitrile
Purity
98%
Packaging
1g
Price
$218
Updated
2021/12/16
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4-hydroxy-3-methylbenzonitrile Chemical Properties,Usage,Production

Synthesis

103264-03-5

15777-70-5

1. Dissolve 4-bromo-2-methylphenol (5.6 g, 30 mmol) and pyridine (6.1 mL, 75 mmol) in 50 mL of anhydrous dichloromethane in an ice bath, and slowly and dropwise add a dichloromethane solution (5 mL) of acetyl chloride (2.8 mL, 26 mmol). After 2 hours of reaction, the reaction mixture was concentrated under reduced pressure. The residue was treated with crushed ice, diluted with 150 mL of dichloromethane, washed with water, dried over anhydrous sodium sulfate, filtered and concentrated under reduced pressure to give 6.9 g of 4-bromo-2-methylphenyl acetate as a light brown oil (quantitative yield). 2. 4-Bromo-2-methylphenyl acetate (6.9 g, 30 mmol) was dissolved in 75 mL of anhydrous dimethylacetamide, zinc cyanide (3 g, 25.6 mmol) and tetrakis(triphenylphosphine)palladium(0) (4.5 g, 3.9 mmol) were added. The reaction mixture was heated at 100 °C for 2 h. After cooling to room temperature, 300 mL of cold water was added. The precipitate was filtered, washed with water and dried over air. Purification by silica gel column chromatography (100% dichloromethane) afforded 5.2 g of 4-cyano-2-methylphenyl acetate as a colorless oil (99% yield), which cured on standing. 3. 4-Cyano-2-methylphenyl acetate (5.2 g, 29.7 mmol) was dissolved in 75 mL of methanol and an aqueous solution (25 mL) of potassium carbonate (30 mmol, 4.15 g) was added. After stirring for 30 min at room temperature, the mixture was concentrated under reduced pressure and treated with 1N sulfuric acid. The precipitate was filtered, washed with water and dried to give 3.1 g of 4-hydroxy-3-methylbenzonitrile as a white solid (78% yield). 4. 4-Hydroxy-3-methylbenzonitrile (3.1 g, 23.3 mmol) was dissolved in 60 mL of anhydrous acetonitrile, cooled to -30 °C, and nitronium tetrafluoroborate (3.4 g, 25.6 mmol) was added in batches. After 60 min of reaction, 100 mL of water was added and diluted. The light yellow precipitate was filtered, washed with water and dried to give 3.9 g of 4-hydroxy-3-methyl-5-nitrobenzonitrile (94% yield). 5. Convert 4-hydroxy-3-methyl-5-nitrobenzonitrile to the target product according to the method for the preparation of 3-fluoro-2-nitrophenyl trifluoromethanesulfonate.

References

[1] Patent: WO2005/30213, 2005, A1. Location in patent: Page/Page column 184
[2] Chemische Berichte, 1891, vol. 24, p. 3671

4-hydroxy-3-methylbenzonitrile Preparation Products And Raw materials

Raw materials

Preparation Products

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4-hydroxy-3-methylbenzonitrile Suppliers

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15777-70-5, 4-hydroxy-3-methylbenzonitrileRelated Search:


  • 4-hydroxy-3-methylbenzonitrile
  • 2-Methyl-4-cyanophenol
  • Benzonitrile, 4-hydroxy-3-methyl-
  • 15777-70-5