ChemicalBook > CAS DataBase List > 9,9-Bis(4-aminophenyl)fluorene

9,9-Bis(4-aminophenyl)fluorene

Product Name
9,9-Bis(4-aminophenyl)fluorene
CAS No.
15499-84-0
Chemical Name
9,9-Bis(4-aminophenyl)fluorene
Synonyms
FDA;BAFL;FDA/BAFL;AKOS BBB/416;Zinc03897005;Anilinefluorene;BIO-FARMA BF003152;TIMTEC-BB SBB008629;9,9-bis(4-aminopheny;bisaminophenylfluorene
CBNumber
CB9439319
Molecular Formula
C25H20N2
Formula Weight
348.44
MOL File
15499-84-0.mol
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9,9-Bis(4-aminophenyl)fluorene Property

Melting point:
237-239 °C (lit.)
Boiling point:
535.2±50.0 °C(Predicted)
Density 
1.245±0.06 g/cm3(Predicted)
storage temp. 
Keep in dark place,Inert atmosphere,Room temperature
Water Solubility 
Insoluble in water
form 
powder to crystal
pka
4.92±0.10(Predicted)
color 
White to Almost white
InChI
InChI=1S/C25H20N2/c26-19-13-9-17(10-14-19)25(18-11-15-20(27)16-12-18)23-7-3-1-5-21(23)22-6-2-4-8-24(22)25/h1-16H,26-27H2
InChIKey
KIFDSGGWDIVQGN-UHFFFAOYSA-N
SMILES
C1(C2=CC=C(N)C=C2)(C2=CC=C(N)C=C2)C2=C(C=CC=C2)C2=C1C=CC=C2
CAS DataBase Reference
15499-84-0(CAS DataBase Reference)
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Safety

Hazard Codes 
Xn,Xi
Risk Statements 
20/21/22-36/37
Safety Statements 
26-36
WGK Germany 
3
HazardClass 
IRRITANT
HS Code 
29215900
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Hazard and Precautionary Statements (GHS)

Symbol(GHS)
Signal word
Warning
Hazard statements

H319Causes serious eye irritation

H335May cause respiratory irritation

Precautionary statements

P261Avoid breathing dust/fume/gas/mist/vapours/spray.

P280Wear protective gloves/protective clothing/eye protection/face protection.

P301+P312IF SWALLOWED: call a POISON CENTER or doctor/physician IF you feel unwell.

P305+P351+P338IF IN EYES: Rinse cautiously with water for several minutes. Remove contact lenses, if present and easy to do. Continuerinsing.

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N-Bromosuccinimide Price

Sigma-Aldrich
Product number
437913
Product name
4,4′-(9-Fluorenylidene)dianiline
Purity
99%
Packaging
25g
Price
$251
Updated
2024/03/01
TCI Chemical
Product number
B1549
Product name
9,9-Bis(4-aminophenyl)fluorene
Purity
>98.0%(T)
Packaging
25g
Price
$110
Updated
2024/03/01
TCI Chemical
Product number
B1549
Product name
9,9-Bis(4-aminophenyl)fluorene
Purity
>98.0%(T)
Packaging
100g
Price
$330
Updated
2024/03/01
TCI Chemical
Product number
B2654
Product name
9,9-Bis(4-aminophenyl)fluorene (purified by sublimation)
Purity
>99.0%(HPLC)(T)
Packaging
1g
Price
$91
Updated
2024/03/01
TRC
Product number
F591593
Product name
4,4''-(9H-Fluorene-9,9-diyl)dianiline
Packaging
2.5g
Price
$90
Updated
2021/12/16
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9,9-Bis(4-aminophenyl)fluorene Chemical Properties,Usage,Production

Description

9,9-Bis(4-aminophenyl)fluorene (FDA) is a fluorene derivative with two aminophenyl substituents on the 9-position. This compound has partial conjugation and can be utilized as a dopant-free organic hole-transporting material in inverted perovskite solar cells. Due to its diaminophenyl groups, FDA is commonly employed in synthesizing polyimides that possess high thermal and hydrolytic stability for optical fiber light guide coatings. Because the FDA is not fully aromatized, it is chosen to produce thermally stable transparent polyimides. Additionally, the polyimide derived from 9,9-bis(4-aminophenyl)fluorene can be further modified through Friedel-Crafts alkylation on the fluorene moiety, as the polyimide backbone remains chemically stable.

Chemical Properties

White powder

Uses

9,9-bis(4-aminophenyl)fluorene be used for preparation of high-strength material and high-temperature polymers.

Preparation

The synthesis of 9,9-Bis(4-aminophenyl)fluorene can be carried out through the following stepwise procedure:
Prepare the reaction mixture:
Place 3.6 g of fluorenone (20 mmol), 7.2 g of aniline hydrochloride (55.6 mmol), 0.5 g of sodium bisulfite (4.8 mmol), 8.8 mL of aniline (96.4 mmol), and 6 mL of toluene in a 100 mL two-necked flask.
Ensure the reaction is conducted under nitrogen protection.
Add a water separator to the two-necked flask.

Begin the reaction:
Stir the reaction mixture and slowly increase the temperature to 120 °C.
Allow the reaction to continue for 30 minutes.
Separate the green liquid produced in the water separator.

Further reaction at elevated temperature:
Continue the reaction at 120 °C for an additional 3 hours.
Separate the water produced in the water separator.

Increase temperature and maintain reaction:
Slowly raise the temperature to 135 °C.
Keep the reaction at this temperature for 1.5 hours.

Monitor for completion:
Check the water separator for any further production of water.
Cease the reaction when no more water is produced in the water separator.

Cool down and adjust pH:
Allow the reacted material to cool to around 60 ℃.
Add 10 wt% potassium hydroxide solution to the reaction mixture.
Adjust the pH of the mixture to 9.
Stir the solution for 15 minutes while it is still hot.

Filtration and purification:
Filter the solution to remove any solid impurities.
Wash the filter cake with water.
Recrystallize the washed filter cake using 30 mL of toluene.
Filter the recrystallized product to obtain pure rice-white product.

Yield determination:
Weigh the obtained pure product, which should amount to 6.55 g.
Calculate the yield by dividing the obtained mass by the theoretical maximum mass and multiplying by 100%.
The yield of the pure rice-white product should be 94%.

General Description

4,4′-(9-Fluorenylidene)dianiline is a diamine.

References

[1] PHAM H D, GIL-ESCRIG L, FERON K, et al. Boosting inverted perovskite solar cell performance by using 9,9-bis(4-diphenylaminophenyl)fluorene functionalized with triphenylamine as a dopant-free hole transporting material?[J]. Journal of Materials Chemistry A, 2019, 20: 12507-12517. DOI:10.1039/C9TA01681C.
[2] G. SONG C. C. Colorless, heat resistant polyimide films derived from 2,3,3′,4′-biphenyltetracarboxylic dianhydride[J]. IOP Conference Series: Materials Science and Engineering, 2020, 73 1. DOI:10.1088/1757-899X/733/1/012035.
[3] WEI J, YU L, YAN L, et al. Synthesis of 9,9-bis(4-hydroxyphenyl) fluorene catalyzed by bifunctional ionic liquids?[J]. RSC Advances, 2021, 52: 32559-32564. DOI:10.1039/D1RA05967J.
[4] SURASAK SEESUKPHRONRARAK. Synthesis and characterization of 9,9-bis(4-hydroxyphenyl and 4-aminophenyl)dibenzofluorenes: Novel fluorene-based monomers[J]. Journal of Polymer Science Part A: Polymer Chemistry, 2019, 57 24: 2602-2605. DOI:10.1002/pola.29540.
[5] HOU CHIEN CHANG. Synthesis of 9,9-bis(4-aminophenyl)fluorene-based benzoxazine and properties of its high-performance thermoset[J]. Journal of Polymer Science Part A: Polymer Chemistry, 2012, 50 11: 2201-2210. DOI:10.1002/pola.25993.
[6] Patent: CN107892649, 2018, A, . Location in patent: Paragraph 0023-0042
[7] Fortschr. Teerfarbenfabr. Verw. Industriezweige, vol. 23, p. 240
[8] DONGHUI YU. Fluorene-Based Phosphine Oxide Host Materials for Blue Electrophosphorescence: An Effective Strategy for a High Triplet Energy Level[J]. Chemistry - A European Journal, 2011, 17 9: 2592-2596. DOI:10.1002/chem.201003434.

9,9-Bis(4-aminophenyl)fluorene Preparation Products And Raw materials

Raw materials

Preparation Products

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9,9-Bis(4-aminophenyl)fluorene Suppliers

HBCChem, Inc.
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View Lastest Price from 9,9-Bis(4-aminophenyl)fluorene manufacturers

Hebei Zhuanglai Chemical Trading Co Ltd
Product
9,9-Bis(4-aminophenyl)fluorene 15499-84-0
Price
US $10.00/kg
Min. Order
1kg
Purity
99%
Supply Ability
20 ton
Release date
2024-11-20
Hebei Chuanghai Biotechnology Co,.LTD
Product
9,9-Bis(4-aminophenyl)fluorene 15499-84-0
Price
US $5.00-2.00/KG
Min. Order
1KG
Purity
99%
Supply Ability
10000kg
Release date
2024-08-23
CHINATECH(TIANJIN) CHEMICAL CO.,LTD.
Product
9,9-Bis(4-aminophenyl)fluorene (FDA) 15499-84-0
Price
US $0.00/Kg/Drum
Min. Order
1KG
Purity
≥99%
Supply Ability
30TM
Release date
2021-12-14

15499-84-0, 9,9-Bis(4-aminophenyl)fluoreneRelated Search:


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