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Terpenes

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Terpenes is the generic term summarizing all kinds of isoprene polymers and their derivatives with its general formula of (C5H8) n. Terpene is a class of compound that is ubiquitous in the plant kingdom, but exist in very few amount in the animal kingdom. Except in the form of terpene hydrocarbons, there are a large number of terpenes forming various kinds of oxygenated derivatives including alcohols, aldehydes, ketones, carboxylic acids, esters and glycoside forms. Secondly there are also nitrogen-containing derivatives as well as a minority of sulfur-containing derivatives presented. Based on the number of the isoprene units contained inside the molecule, the terpenes can be divided into: monoterpene, sesquiterpenoid, diterpene, sesquiterpene, triterpenoids, tetraterpene and polyterpene.

For some compound which originated from the synthesis of isoprene, but has the number of carbon atoms in the molecule be not an integer multiple of 5, they are called terpenoid. In the life activities, terpenoids compound, especially inside the plants, have important functions, for example gibberellin, abscisic acid and insect juvenile hormone are important hormones, carotenoids and chlorophyll are important photosynthetic pigments; plastoquinone and quinone are respectively important electronic chain delivery body in photosynthesis and respiration chain; sterols are the component of the biological membrane.

Monoterpene and sesquiterpene are the major component of volatile oil. Diterpene is the major substance forming the resin; triterpenoid is an important material forming plant saponins and resins, tetraterpene mainly include some fat-soluble pigments widely distributed in the plants. In nature, terpenoids is widely distributed, some of which have physiological activity. For example, ascaridole and santonin have roundworm expelling effect; artemisinin has antimalarial effect while andrographolidume has antibacterial effect.

The following describes some of the chemical reactions associated with terpenes. This is significant for determination of the chemical structure of terpene component.

(1) Oxidation reaction
Different oxidants, in different situations, can oxidize the different groups contained in terpene component to produce different products. For example, chromic acid can oxidize the carbon methyl group and gem-dimethyl carbon to produce acetic acid; the oxidation reaction of ozone is a valuable double bond cleavage reaction and can determine the position of double bond in the structure of the terpene composition. Lead tetraacetate is also oxidation agents of double-bond and has been widely used in chemical research of the terpene ingredients.

(2) The dehydrogenation
Dehydrogenation reaction can be considered as a kind of oxidation reactions and is a kind of valuable reaction for the study the chemical structure of terpenes particularly cyclic terpene. It refers to that the terpene component is heated (200 ℃ ~ 300 ℃) together with sulfur or selenium under an inert atmosphere, the carbon skeleton of the cyclic terpene is dehydrogenated into aromatic derivatives with sometimes the ring being cleaved and sometimes cyclization occurring simultaneously.

(3) Addition reaction
The double bonds in the terpene components can react with hydrogen halide acids such as hydroiodic acid or hydrogen chloride in glacial acetic acid solution to generate crystalline-shaped addition product. It can also absorb bromine (diethyl ether or glacial acetic acid - ethanol solution) to generate bromide with certain physicochemical properties. If mixing the glacial acetic acid and sodium nitrite for shaking, nitrous oxide or pseudo-nitrous oxide will be generate and will exhibit visible special colors.
If the unsaturated terpene component was added with amyl nitrite and concentrated hydrochloric acid for mixing with shaking and keep it cool, then add a small amount of ethanol or glacial acetic acid, there will be chlorinated nitroso derivative of terpenes generated with special colors as well. Such nitroso derivatives (including nitrous oxides and chlorinated nitroso derivative) mostly exhibit blue or blue-green color. They are easily polymerized to form a colorless di-polymer, but when the di-polymer is heated to a molten state or when made into a solution, it can also be converted into a blue or blue-green single-molecule compound.
Nitroso chlorinated derivatives can condense with primary or secondary amines (commonly piperidine) to generate nitroso amines with most of them having complete crystal shape and  certain physical and chemical constants available for the identification of unsaturated terpene components. If the terpene component molecules contain conjugated double bonds, then it will form crystalline addition product with maleic anhydride through Diels-Alder reaction which can be used to prove the presence of conjugated double bonds.

(4) Wagner-Meerweein rearrangement;
Terpene molecules, sometimes through the effect of agents (such as acid, etc.), the carbon skeleton can be changed or the functional groups in the molecule can be transferred in the molecule. Especially during the elimination reaction, addition reaction or a nucleophilic substitution reaction of bicyclic terpene compound, there is often Wagner-Meerweein rearrangement happening.

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Structure:
Chemical Name:
ent-6,9-Dihydroxy-15-oxo-16-kauren -19-oic acid beta-D-glucopyrasyl ester
CAS:
81263-98-1
MF:
C26H38O10
Structure:
Chemical Name:
ent-kaurane-3,16,17-triol
CAS:
130855-22-0
MF:
C20H34O3
Structure:
Chemical Name:
Esculentic acid
CAS:
103974-74-9
MF:
C30H48O5
Structure:
Chemical Name:
Isocoronarin D
CAS:
138965-88-5
MF:
C20H30O3
Structure:
Chemical Name:
11beta-Hydroxycedrelone
CAS:
283174-18-5
MF:
C26H30O6
Structure:
Chemical Name:
9(11),12-Oleanadien-3-ol
CAS:
94530-87-7
MF:
C30H48O
Structure:
Chemical Name:
Abiesadine N
CAS:
1159913-80-0
MF:
C21H30O3
Structure:
Chemical Name:
Aglinin A
CAS:
246868-97-3
MF:
C30H50O5
Structure:
Chemical Name:
1-O-Deacetylkhayalide E
CAS:
1007387-95-2
MF:
C27H32O10
Structure:
Chemical Name:
2,16-Kauranediol
CAS:
34302-37-9
MF:
C20H34O2
Structure:
Chemical Name:
2,6-Dimethyl-3,7-octadiene-2,6-diol
CAS:
51276-34-7
MF:
C10H18O2
Structure:
Chemical Name:
20-Hydroxy-3-oxo-28-lupaic acid
CAS:
93372-87-3
MF:
C30H48O4
Structure:
Chemical Name:
24,25-Epoxy-dammar-20(21)-en-3-one
CAS:
63543-52-2
MF:
C30H48O2
Structure:
Chemical Name:
3-Hydroxylast-9(11),24-dien-26-oic acid
CAS:
129724-83-0
MF:
C30H48O3
Structure:
Chemical Name:
(24E)-3-Oxo-5α-lanosta-7,9(11),24-trien-26-oic acid
CAS:
104759-35-5
MF:
C30H44O3
Structure:
Chemical Name:
(13α,14β,17α,20R)-22,25-Epoxy-23,24-dihydroxy-5α-lanost-7-en-3-one
CAS:
16962-90-6
MF:
C30H48O4
Structure:
Chemical Name:
(5E,9E,13E,17E,21E,25E,29E)-6,10,14,18,22,26,30,34-Octamethyl-5,9,13,17,21,25,29,33-pentatriacontaocten-2-one
CAS:
21978-49-4
MF:
C43H70O
Structure:
Chemical Name:
(2R,3aα,5aα,6aβ,10bβ,10cα)-9α-(3-Furyl)dodecahydro-2β-hydroxy-10aα-methyl-4H,7H-furo[2',3',4':4,5]naphtho[2,1-c]pyran-4,7-dione
CAS:
67567-15-1
MF:
C19H22O6
Structure:
Chemical Name:
Glochidone
CAS:
6610-55-5
MF:
C30H46O
Structure:
Chemical Name:
ent-6,9-Dihydroxy-15-oxo-16-kauren-19-oic acid
CAS:
81264-00-8
MF:
C20H28O5
Structure:
Chemical Name:
Isotschimgin
CAS:
62356-47-2
MF:
C17H22O3
Structure:
Chemical Name:
Liangshanin A
CAS:
122717-54-8
MF:
C20H26O4
Structure:
Chemical Name:
Masticadielic acid
CAS:
472-30-0
MF:
C30H48O3
Structure:
Chemical Name:
Methylpseudolarate B
CAS:
82508-34-7
MF:
C24H30O8
Structure:
Chemical Name:
Momethyl kolavate
CAS:
24513-41-5
MF:
C21H32O4
Structure:
Chemical Name:
Ohchinin acetate
CAS:
67023-81-8
MF:
C38H44O9
Structure:
Chemical Name:
Simiarene
CAS:
2318-78-7
MF:
C30H48O
Structure:
Chemical Name:
Tetrahydroxysqualene
CAS:
1043629-23-7
MF:
C30H50O4
Structure:
Chemical Name:
15,16-Dihydro-15-Methoxy-16-oxohardwickiic acid
CAS:
115783-35-2
MF:
C21H30O5
Structure:
Chemical Name:
3,27-Dihydroxy-20(29)-lupen-28-oic acid Methyl ester
CAS:
263844-79-7
MF:
C31H50O4
Structure:
Chemical Name:
14-Deoxy-11,12-didehydroandrographiside
CAS:
141973-41-3
MF:
C26H38O9
Structure:
Chemical Name:
3,10-Dihydroxy-5,11-dielMenthadiene-4,9-dione
CAS:
106623-23-8
MF:
C20H28O4
Structure:
Chemical Name:
Quinovic acid 3-O-alpha-L-rhaMnopyranoside
CAS:
104055-76-7
MF:
C36H56O9
Structure:
Chemical Name:
ZEORINE
CAS:
22570-53-2
MF:
C30H52O2
Structure:
Chemical Name:
Trichokaurin
CAS:
23811-50-9
MF:
C24H34O7
Structure:
Chemical Name:
mupinensisone
CAS:
152253-67-3
MF:
C30H48O2
Structure:
Chemical Name:
14-deoxyandrographoside
CAS:
82209-72-1
MF:
C26H40O9
Structure:
Chemical Name:
Oleanolic acid 3-acetate
CAS:
4339-72-4
MF:
C32H50O4
Structure:
Chemical Name:
24-methylene cycloartanol
CAS:
1449-09-8
MF:
C31H52O
Structure:
Chemical Name:
LIMONOL
CAS:
989-61-7
MF:
C26H32O8
Structure:
Chemical Name:
Nodosin
CAS:
10391-09-0
MF:
C20H26O6
Structure:
Chemical Name:
Picrasil B
CAS:
89498-91-9
MF:
C22H32O6
Structure:
Chemical Name:
Sculponeatic acid
CAS:
1169806-02-3
MF:
C30H46O4
Structure:
Chemical Name:
Spiramilactone B
CAS:
180961-65-3
MF:
C20H26O4
Structure:
Chemical Name:
Triptohypol F
CAS:
268541-26-0
MF:
C31H52O2
Structure:
Chemical Name:
Xerophilusin G
CAS:
304642-94-2
MF:
C22H30O8
Structure:
Chemical Name:
21,24-Epoxycycloartane-3,25-diol
CAS:
125305-73-9
MF:
C30H50O3
Structure:
Chemical Name:
27-HydroxyMangiferolic acid
CAS:
17983-82-3
MF:
C30H48O4
Structure:
Chemical Name:
3-Epiglochidiol diacetate
CAS:
6587-37-7
MF:
C34H54O4
Structure:
Chemical Name:
Bisandrographolide A
CAS:
160498-00-0
MF:
C40H56O8
Structure:
Chemical Name:
CycloMusalenone
CAS:
30452-60-9
MF:
C30H48O
Structure:
Chemical Name:
Pterokaurene L3
CAS:
77658-38-9
MF:
C20H30O3
Structure:
Chemical Name:
IsoMangiferolic acid
CAS:
13878-92-7
MF:
C30H48O3
Structure:
Chemical Name:
14-Deoxycoleon U
CAS:
88664-09-9
MF:
C20H26O4
Structure:
Chemical Name:
pinusolide
CAS:
31685-80-0
MF:
C21H30O4
Structure:
Chemical Name:
Baccatin VI
CAS:
57672-79-4
MF:
C37H46O14
Structure:
Chemical Name:
11α-Acetoxy-7α,20-epoxy-6β,7-dihydroxykaur-16-en-15-one
CAS:
77949-42-9
MF:
C22H30O6
Structure:
Chemical Name:
(13S)-10-Demethyl-9α-methylpimarane-5α,15,16-triol
CAS:
7121-99-5
MF:
C20H36O3
Structure:
Chemical Name:
Lup-20(29)-ene-1β,3β-diol
CAS:
29028-10-2
MF:
C30H50O2
Structure:
Chemical Name:
(20S,24S)-20,24-Epoxydammarane-3β,25-diol
CAS:
19942-04-2
MF:
C30H52O3
Structure:
Chemical Name:
14-Isopropylpodocarpa-8,11,13-triene-3β,13-diol
CAS:
3772-56-3
MF:
C20H30O2
Structure:
Chemical Name:
(4S)-4α-[(Z)-2-(3-Furyl)vinyl]-4a,5,6,7,8,8aβ-hexahydro-3,4aα,8,8-tetramethylnaphthalen-1(4H)-one
CAS:
56324-54-0
MF:
C20H26O2
Structure:
Chemical Name:
(1S)-2α,5α-(Epoxymethano)-1-hydroxymethyl-2-(2-hydroxyethyl)cyclopentan-1β-ol
CAS:
126594-66-9
MF:
C9H16O4
Structure:
Chemical Name:
13-Methyl-8,11,13-podocarpatriene-3,12-diol
CAS:
769140-74-1
MF:
C18H26O2
Structure:
Chemical Name:
1-O-Deacetyl-2alpha-hydroxykhayalide E
CAS:
1189801-51-1
MF:
C27H32O11
Structure:
Chemical Name:
2,16,19-Kauranetriol 2-O-beta-D-allopyraside
CAS:
195723-38-7
MF:
C26H44O8
Structure:
Chemical Name:
2,6,16-Kauranetriol 2-O-beta-D-allopyraside
CAS:
195735-16-1
MF:
C26H44O8
Structure:
Chemical Name:
24,25-Dihydroxydammar-20-en-3-one
CAS:
63543-53-3
MF:
C30H50O3
Structure:
Chemical Name:
3-Hydroxy-12-oleanene-23,28-dioic acid
CAS:
226562-47-6
MF:
C30H46O5
Structure:
Chemical Name:
Abiesadine I
CAS:
1210347-50-4
MF:
C24H34O5
Structure:
Chemical Name:
Agathadiol diacetate
CAS:
24022-13-7
MF:
C24H38O4
Structure:
Chemical Name:
Deacetylpseudolaric acid A
CAS:
82508-37-0
MF:
C20H26O5
Structure:
Chemical Name:
ent-6,11-Dihydroxy-15-oxo-16-kauren -19-oic acid beta-D-glucopyrasyl ester
CAS:
81263-97-0
MF:
C26H38O10
Structure:
Chemical Name:
Erythrodiol 3-palmitate
CAS:
19833-13-7
MF:
C46H80O3
Structure:
Chemical Name:
Kamebanin
CAS:
39388-57-3
MF:
C20H30O4
Structure:
Chemical Name:
Sorghumol acetate
CAS:
90582-47-1
MF:
C32H52O2
Structure:
Chemical Name:
Tanshinlactone
CAS:
105351-70-0
MF:
C17H12O3
Structure:
Chemical Name:
Uncargenin C
CAS:
152243-70-4
MF:
C30H48O5
Structure:
Chemical Name:
Zamanic acid
CAS:
260393-05-3
MF:
C39H54O6
Structure:
Chemical Name:
14-Deoxy-17-hydroxyandrographolide
CAS:
869384-82-7
MF:
C20H32O5
Structure:
Chemical Name:
4-EpicoMMunic acid
CAS:
83945-57-7
MF:
C20H30O2
Structure:
Chemical Name:
Ursonic acid
CAS:
6246-46-4
MF:
C30H46O3
Structure:
Chemical Name:
(1alpha,4alpha,6alpha)-(±)-1,3,3-trimethyl-2-oxabicyclo[2.2.2]octan-6-ol
CAS:
60761-00-4
MF:
C10H18O2
Structure:
Chemical Name:
(4aS,10aS)-6-hydroxy-1,1,4a-trimethyl-7-propan-2-yl-3,4,10,10a-tetrahy dro-2H-phenanthren-9-one
CAS:
511-05-7
MF:
C20H28O2
Structure:
Chemical Name:
nagilactone C
CAS:
24338-53-2
MF:
C19H22O7
Structure:
Chemical Name:
rehmannic acid
CAS:
467-81-2
MF:
C35H52O5
Structure:
Chemical Name:
psi-taraxasterol
CAS:
464-98-2
MF:
C30H50O
Structure:
Chemical Name:
3α,20-Dihydroxy-4,4,14-trimethyl-18-nor-5α-cholan-24-oic acid γ-lactone
CAS:
35833-72-8
MF:
C27H44O3
Structure:
Chemical Name:
(24R)-20,24-Epoxy-25-hydroxy-3,4-seco-5α-dammar-4(28)-en-3-oic acid
CAS:
21671-00-1
MF:
C30H50O4
Structure:
Chemical Name:
(24Z)-3,4-Secolanosta-4(28),9(11),24-triene-3,26-dioic acid
CAS:
62393-88-8
MF:
C30H46O4
Structure:
Chemical Name:
(13S,14S,17S)-3,6-Dioxo-16β-hydroxylanosta-7,24-diene-21-oic acid γ-lactone
CAS:
64929-59-5
MF:
C30H42O4
Structure:
Chemical Name:
1,2,3,19-Tetrahydroxy-12-ursen-28-oic acid
CAS:
113558-03-5
MF:
C30H48O6
Structure:
Chemical Name:
11,15-Dihydroxy-16-kauren-19-oic acid
CAS:
57719-76-3
MF:
C20H30O4
Structure:
Chemical Name:
13-O-Deacetyltaxumairol Z
CAS:
220935-39-7
MF:
C31H40O12
Structure:
Chemical Name:
16-Hydroxy-8(17),13- labdadien-15,16-olid-19-oic acid
CAS:
691009-85-5
MF:
C20H28O4
Structure:
Chemical Name:
22-Hydroxy-3-oxo-12-ursen-30-oic acid
CAS:
173991-81-6
MF:
C30H46O4
Structure:
Chemical Name:
Alstonic acid B
CAS:
1159579-45-9
MF:
C30H46O3
Structure:
Chemical Name:
Coronalolic acid
CAS:
268214-52-4
MF:
C30H46O4
Structure:
Chemical Name:
Daturabietatriene
CAS:
65894-41-9
MF:
C20H30O2
Structure:
Chemical Name:
Dihydroajugapitin
CAS:
87480-84-0
MF:
C29H44O10